Advanced Search
  • Included in CSCD
  • Chinese Core Journals
  • Included in WJCI Report
  • Included in Scopus, CA, DOAJ, EBSCO, JST
  • The Key Magazine of China Technology
Volume 38 Issue 1
Feb.  2019
Turn off MathJax
Article Contents
Article Navigation >  CARSOLOGICA SINICA  > 2019  >  38(1): 19-27
LI Yang, YANG Zhen, KANG Fengxin, LIU Jinyong, SUN Yanwei, HUANG Jingbo. Isotope analysis on the source of nitrate contamination to groundwater in the Dong’e hydrogeologic unit[J]. CARSOLOGICA SINICA, 2019, 38(1): 19-27. doi: 10.11932/karst20190103
Citation: LI Yang, YANG Zhen, KANG Fengxin, LIU Jinyong, SUN Yanwei, HUANG Jingbo. Isotope analysis on the source of nitrate contamination to groundwater in the Dong’e hydrogeologic unit[J]. CARSOLOGICA SINICA, 2019, 38(1): 19-27. doi: 10.11932/karst20190103
shu

Isotope analysis on the source of nitrate contamination to groundwater in the Dong’e hydrogeologic unit

doi: 10.11932/karst20190103
  • 1.

    Shandong Geophysical and Geochemical Exploration Institute, Jinan, Shandong 250013 ，China/Shandong Soil Geochemical Engineering Laboratery, Jinan, Shandong 250013 , China

  • 2.

    Shandong Geophysical and Geochemical Exploration Institute, Jinan, Shandong 250013 ，China

  • 3.

    Shandong Bureau of Geology&Mineral Resources,Jinan,Shandong 250013 , China

  • Publish Date: 2019-02-25
    Abstract
  • In recent years, nitrate pollution to groundwater has been increasingly serious, In this work, nitrogen isotope technique was used to study such pollution in a typical agricultural area of the Dong’e hydrogeological unit. The results show that the content of NO3- at monitoring sites of shallow groundwater is high with average content of 27.77 mg·L-1; and the content of δ15N is between 7.8‰ to 12‰, indicating the shallow groundwater is contaminated by sewage or feces. NO3- content of deep groundwater (karst water) is relatively low with an average value 12.81 mg·L-1, and the content of δ15N is in 7.2‰-14.3‰ also indicating sewage or fecal contamination, closely related to human disturbance. The groundwater quality of some monitoring sites is poor. It is suggested that efficient irrigation technology and scientific fertilization should be used in the study area, poultry farms can be built through fermentation tanks and improved feed formulations, thus to reduce the exogenous input of groundwater nitrate from the source.

     

    • FullText(HTML)
  • loading
    • References(28)
  • [1]
    Wang J L, Yang Y S. An approach to catchment-scale groundwater nitrate risk assessment from diffuse agricultural sources: A case study in the Upper Bann, Northern Ireland［J］. Hydrological Processes, 2008, 22(21):4274-4286.
    [2]
    Nixdorf E, Sun Y Y, Lin M, et al. Development and application of a novel method for regional assessment of groundwater contamination risk in the Songhua River Basin［J］. Science of The Total Environment, 2017, 605:598-609.
    [3]
    Jones R R , Weyer P J , Dellavalle C T , et al. Nitrate from Drinking Water and Diet and Bladder Cancer Among Postmenopausal Women in Iowa［J］. Environmental Health Perspectives, 2016, 124(11):1751-1758.
    [4]
    Li P Y, Li X Y, Meng X Y, et al. Appraising Groundwater Quality and Health Risks from Contamination in a Semiarid Region of Northwest China［J］. Exposure & Health, 2016, 8(3):361-379.
    [5]
    杨淡，蔡鹤生，刘存富，等. NO3中15N和18O同位素新技术在岩溶地区地下水氮污染研究中的应用—以河南林州食管癌高发区研究为例［J］.中国岩溶,2004,23(3):206- 212.
    [6]
    Colin M W.US report raises fears over nitrate levels in water［J］.Nature,1995,377:4.
    [7]
    张翠云, 王昭, 程旭学. 张掖市地下水硝酸盐污染源的氮同位素研究［J］.干旱区资源与环境,2004,18(1):79-85.
    [8]
    刘宏斌, 张云贵, 李志宏, 等. 北京市平原农区深层地下水硝态氮污染状况研究［J］.土壤学报,2005,42(3):411-418.
    [9]
    乔光建, 张均玲, 唐俊智.地下水氮污染机理分析及治理措施［J］.水资源保护,2004,20(3):9-12.
    [10]
    Kendall C, McDonnell JJ. Isotope tracers in catchment hydrology［J］. Elsevier Science，1998, 519-569.
    [11]
    Spalding R F, Z. K U, Hyun S W, et al. Source identification of nitrate on Cheju Island, South Korea［J］. Nutrient Cycling in Agroecosystems, 2001, 61(3):237-246.
    [12]
    Choi W J, Yoon K S, Ro H M, et al. Impact of landuse types on nitrate concentration and δ15N in unconfined groundwater in rural areas of Korea［J］. Agriculture Ecosystems & Environment, 2007, 120(2):259-268.
    [13]
    Fryar A E, Macko S A, Iii W F M, et al. Nitrate reduction during ground-water recharge, Southern High Plains, Texas［J］. Journal of Contaminant Hydrology, 2000, 40(4):335-363.
    [14]
    Krotkiewski H, Duk M, Syper D, et al. Intermittent denitrification: The application of a 15N natural abundance method to a forested ecosystem［J］. Geochimica et Cosmochimica Acta, 1997, 61(23):5043-5050.
    [15]
    李思亮,刘丛强,肖化云,等.δ15N在贵阳地下水氮污染来源和转化过程中的辨识应用［J］.地球化学，2005,34(3):257-262.
    [16]
    庞会从，刘福亮，付海燕，等. 2009-2014 年河北平原浅层地下水硝态氮特征及其来源［J］.环境工程学报，2015,9（10）：4766-4772.
    [17]
    张翠云，张胜，李政红，等. 利用氮同位素技术识别石家庄市地下水硝酸盐污染源［J］.地球科学进展，2004,19（2）：183-190.
    [18]
    吴登定，姜月华，贾军远，等.运用氮、氧同位素技术判别常州地区地下水氮污染源［J］. 水文地质工程地质，2007,3:15-15.
    [19]
    黄强盛，李清光，卢玮琦，等.滇池流域地下水、河水硝酸盐污染及来源［J］. 地球与环境，2014,42（5）:589-596
    [20]
    Singleton M J, Woods K N, Conrad M E, et al. Tracking Sources of Unsaturated Zone and Groundwater Nitrate Contamination Using Nitrogen and Oxygen Stable Isotopes at the Hanford Site, Washington［J］. Environmental Science & Technology, 2005, 39(10):3563-3570.
    [21]
    Sacchi E, Acutis M, Bartoli M, et al. Origin and fate of nitrates in groundwater from the central Po plain: Insights from isotopic investigations［J］. Applied Geochemistry, 2013, 34:164-180.
    [22]
    Heaton THE. Isotopic studies of nitrogen pollution in the hydrosphere and atmosphere: A review ［J］. Chemical Geology, 1986, 59: 87-1021.Heaton T H E . Isotopic studies of nitrogen pollution in the hydrosphere and atmosphere: A review［J］. Chemical Geology, 1986, 59(2):87-102.
    [23]
    Wassenaar L. Evaluation of the origin and fate of nitrate in the Abbotsford aquifer using the isotopes of 15N and 18O in NO3［J］. Applied Geochemistry, 1995, 10: 391-405.
    [24]
    Korotkevich A Y , Kuznetsova N A , Tiunov A V . Changes in carbon and nitrogen isotope ratios (13C/12C and 15N/14N) in springtails during long-term storage of soil samples［J］. Russian Journal of Ecology, 2016, 47(6):572-574.
    [25]
    丁京涛, 席北斗, 许其功, 等. 稳定同位素技术在地表水硝酸盐污染研究中的应用［J］. 湖泊科学, 2013,25（5）：617-627.
    [26]
    Xue D M, Botte J, Baets B D, et al. Present limitations and future prospects of stable isotope methods for nitrate source identification in surface-and groundwater［J］. Water Research, 2009, 43(5):1159-1170.
    [27]
    宋晓焱, 尹国勋, 谭利敏, 等. 污水灌溉对地下水污染的机理研究［J］.安全与环境学报，2006,6（1）：136-138.
    [28]
    王玉强. 上海市域地下水环境氯离子含量的时空演化特征研究［J］.山东农业大学学报(自然科学版),2015,46(6):892-897.
    • Relative Articles
    • Supplements(0)
    • Cited By
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF(4932.0KB)
    XML

    Article Metrics

    Article views (1990) PDF downloads(590) Cited by()
    Proportional views
    Related

    Website Copyright © CARSOLOGICA SINICA 桂ICP备05009877号-1

    Sponsor: Chinese Academy of Geological Sciences Sponsored by: Institute of Karst Geology, Chinese Academy of Geological Sciences Address: No.50, Qixing Road, Guilin, Guangxi

    Post Code: 541004 Tel: 0773-5812949 7796657 Email: zgyr@mail.cgs.gov.cn; zgyrbjb@163.com

    Supported by: Beijing Renhe Information Technology Co., Ltd.    

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return